The main objective of this study was to use an uncertainty version of a widely used monthly time step, semi-distributed model (the Pitman model) to explore the equifinalities in the way in which the main hydrological processes are simulated and any identifiable linkages with uncertainties in the available observational data. The study area is the Zambezi River basin and 18 gauged sub-basins have been included in the analyses. Unfortunately, it is not generally possible to quantify some of the observational uncertainties in such a data scarce area and mostly we are limited to identifying where these data are clearly deficient (i.e. erroneous or non-representative). The overall conclusion is that the equifinalities in the model are hugely dominant in terms of the uncertainties in the relative occurrence of different runoff generating processes, although water use uncertainties in the semi-arid parts of the basin can contribute to these uncertainties. The identification of landscape features that suggest the occurrence of saturation excess surface runoff provides some information to constrain the model. Improved independent estimates of groundwater recharge is also identified as a key source of observational data that would help a great deal in constraining the model parameter space and therefore reducing some of the model equifinality.