In this paper, we discuss the existence of $IS$-asymptotically $\omega$-periodic mild L-quasi-solutions for a class of fractional evolution equations with non-instantaneous impulses. Under a new concept of upper and lower solutions, a new monotone iterative technique is constructed, and the necessary conditions for the existence of extremal coupled mild $L$-quasi-solutions are obtained. Finally, an example is given to illustrate the effectiveness of our theoretical results.