Developing channel models typically requires aggregating channel measurements and the corresponding extracted propagation parameters from different research institutions to form a sufficiently large data basis. However, uncertainties arising from limitations of the sounding hardware and algorithms may greatly impact the comparability between sounding results. Especially, (sub-) THz channel sounding is challenged by a potentially low SNR. At the same time, high Doppler shifts may occur due to the high carrier frequencies, limiting the time spans for coherent or incoherent data processing. Hence, the channel dynamics additionally restrict the processing gain for the SNR. In this paper, we address these challenges metrologically from several perspectives. First, we discuss methods of baseband waveform precoding to adapt it to the sounder hardware or the employed high-resolution estimation algorithms. This allows using available transmit power in an optimal sense. Second, the assessment of the sounder performance requires a traceable reference allowing tracing back measurements (or estimated propagation parameters) to a physical ground truth. Therefore, we propose and discuss an over-the-air artifact allowing a joint verification of delay and Doppler parameters in a multipath scenario. The evaluations of exemplary sub-THz measurements with a multicarrier-based sounder highlight the strong interplay between sounder hardware and estimation algorithms, especially when coping with the mutual interference of parameters from multiple propagation paths. Hence, a metrological assessment always requires considering the full processing pipeline from the unprocessed measurements up to the extracted propagation parameters.