The Asian Summer Monsoon (ASM) has garnered attention in recent years for its impacts on the composition of the upper troposphere and lower stratosphere (UTLS) via deep convection. A recent observational effort into this mechanism, the Asian summer monsoon Chemical and CLimate Impact Project (ACCLIP), sampled the composition of the ASM UTLS over the northwestern Pacific during boreal summer 2022 using two airborne platforms. In this work, we integrate Lagrangian trajectory modeling with convective cloud top observations to diagnose ASM convective transport which contributed to ACCLIP airborne observations. This diagnostic is applied to explore the properties of convective transport associated with prominent ASM sub-systems, revealing that convective transport along the East Asia Subtropical Front generally contained more pollutants than from South Asia, for species ranging in lifetime from days to months. The convective transport diagnostic is used to isolate three convective transport events over eastern Asia which had distinct chemical tracer relationship slopes, indicating the different economical behaviors of the contributing source regions. One of these transport events is explored in greater detail, where a polluted air mass was sampled from convection over the Northeast China Plain. This event was largely confined to 12-15 km altitude, which may be high enough to impact the composition of the stratosphere. Overall, the presented diagnosis of convective transport contribution to ACCLIP airborne sampling indicates a key scientific success of the campaign and enables process studies of the climate interactions from the two ASM sub-system.

COVID-19’s impact on society and our daily habits has been unprecedented. With a decrease in vehicular traffic and industrial production, a decrease in local emissions was expected to occur. In order to capture any trends in ambient trace gas concentrations, approximately one thousand whole air samples were collected in intervals across the United States from April to July 2020 as part of the NASA Student Airborne Research Program (SARP). These samples were then analyzed by the UCI Rowland-Blake Lab using multi-column gas chromatography for over one hundred unique trace gases, including methane, non-methane hydrocarbons, and halocarbons, as described in Colman et al. (2001) and Barletta et al. (2002). Initial samples collected in April coincided with the peak of stay-at-home/social distancing orders in most states while samples collected later in the spring and early summer reflect the easing of these measures and initial state reopenings. Overall trends in emissions over time in select metropolitan areas will be discussed and compared to trends observed across the entire United States.

The 2020 COVID-19 pandemic provided a unique opportunity to sample atmospheric gases during a period of very low industrial/human activity. Over 1000 Whole Air Samples were collected in over 30 cities and towns across the United States from April through July 2020 as part of the NASA Student Airborne Research Program (SARP). Sample locations leveraged the geographic distribution across the United States of the undergraduate and graduate students, faculty, and NASA personnel associated with the internship program (44 people total). Each person collected approximately 24 air samples in their city/town with the goal of characterizing local emissions with time during the pandemic. Samples were collected in 2-Liter stainless steel evacuated canisters at approximately 2 meters above ground level. The canisters were shipped to the Rowland/Blake Laboratory at the University of California Irvine and analyzed for methane, carbon dioxide, carbon monoxide, non-methane hydrocarbons, and halocarbons using the gas chromatographic system described in Colman et al. (2001) and Barletta et al. (2002). Initial samples collected in April coincided with the peak of stay-at-home/social distancing orders across most of the United States while samples collected later in the spring and early summer reflect the easing of these measures in most locations. Overall trends in emissions with time across the United States during the pandemic (in several large metro areas as well as rural locations) will be discussed.