We use the hydrological model WaterGAP v2.2e in the range 1901-2019 and with climate forcing and including the direct human impacts to calculate the hydrologically-induced perturbations in the Earth's axial moment of inertia and rotation rate of the mantle, thereby deriving deviations in Length of Day (∆LOD) from the nominal 86,400 seconds. We present 10 individual components of this Terrestrial Water Storage (TWS), namely, water storage in canopies, snow, soil, groundwater, local lakes, global lakes, local wetlands, global wetlands, reservoirs, and rivers. We show that changes in snowfall patterns and melting of glaciers under climate change, groundwater usage due to direct human influence, as well as impoundment of reservoirs, are the three most important long-term contributors, exhibiting trends as large as 0.19 milliseconds per century. However, we argue that there are discrepancies between this trend and that derived from satellite gravimetry, thus revealing the unaccounted contribution of polar ice sheets. We demonstrate the consistency of our estimates with independent series generated by GFZ German Research Center for Geosciences in the range 1976-2019. In addition, by comparing our results with the observed ∆LOD from space geodesy, we explain a considerable portion of this observed signal on seasonal to interannual timescales. Our results provide daily hydrological excitations of ∆LOD, extending the temporal range of the currently available excitation series to the early 20 th century and including individual contributors to TWS under climate change and direct human influence. This proves useful in better constraining other important contributors to ∆LOD, particularly the core dynamics.