The Atmospheric Radiation Measurement (ARM) Data Center (ADC), at Oak Ridge National Laboratory (ORNL), is a central hub of the U.S. Department of Energy’s ARM user facility and supports global climate and atmospheric science by managing one of the most comprehensive and openly accessible archives of atmospheric observations in the world. With over seven petabytes of curated data spanning more than 30 years, the ADC processes and distributes over 50 terabytes of new data each month from fixed, mobile, and aerial observatories operating in climate-critical regions worldwide.As data grows in volume, complexity, and value, the ADC is advancing new AI- and ML-enabled capabilities to transform how users discover, access, and interact with ARM data. These efforts align with broader DOE and ORNL initiatives in building scalable, FAIR-aligned (Findable, Accessible, Interoperable, and Reusable) data ecosystems supporting the next generation of open science.Central to this transformation are AI-powered, user-centric tools that assist researchers through natural language interfaces, simplifying the process of identifying relevant data products across ARM’s complex metadata hierarchies. These tools reduce the entry barrier for new users while enabling personalized discovery pathways for more experienced users. By bridging and translating across diverse metadata structures, these tools enhance data usability and streamline cross-domain discovery. These tools also leverage a scalable vector-based infrastructure that enables contextual understanding, user-aware recommendations, and integration into future AI-ready APIs.The ADC’s broader portfolio includes AI-powered metadata and abstract generation, anomaly and epoch detection models, a Primary Measurement Type classifier, and a data recommendation engine – each advancing automation, knowledge extraction, and scalable ML pipeline readiness. Strategic collaborations with the USGS, the Earth Science Information Partners (ESIP), and ORNL’s AI Program further strengthen these efforts to accelerate AI-driven workflows. Together, these efforts position the ADC at the forefront of intelligent Earth science data platforms and open science innovation, enabling intuitive, efficient and more impactful scientific discovery.