Peatlands cover approximately three percent of Earthâs land surface, sequestering roughly one-third of terrestrial carbon while releasing nearly ten percent of atmospheric methane on an annual basis. Shifts in global temperature can alter these landscapes, from storing carbon under cold and waterlogged conditions, to rapidly expelling carbon during warmer and drier periods. In this study, we use eddy covariance datasets from the AmeriFlux Network (Lawrence Berkeley National Laboratory) to explore statistically significant spatial and temporal relationships between atmospheric variables and carbon fluxes, across two northern peatland systems with distinct hydrologic regimes: the Bonanza Creek Thermokarst Bog in Alaska, USA, and the Marcell Bog Lake Fen in Minnesota, USA. We set up a generalized multi-site long short-term memory (LSTM) model, trained on atmospheric and flux data, from four sites in Alaska in an effort to estimate methane fluxes at a fifth site, Bonanza Creek, using only atmospheric variables as inputs. For Marcell Bog Lake, we trained a complementary LSTM using a sequential 80:20 trainâtest split for estimation and evaluation. Half-hourly data from 2010 to 2020 was used for statistical analysis and to train each model. On average, Spearman correlation coefficients (Ď) revealed a subtle inverse relationship for methane flux and atmospheric pressure in winter months (Ď=-0.21), with considerable variability observed in spring and summer. Stronger positive correlations were shown for methane flux and air temperature (Ď=0.46), which remained relatively consistent across the four seasons. This was also apparent for methane concentration and humidity (Ď=0.58), suggesting that more saturated air tended to be associated with elevated methane levels. While overall model performance reflects the inherent challenges of cross-site prediction, the LSTM results exhibit a strong temporal agreement with flux observations for Bonanza Creek and Marcell Bog Lake, respectively, demonstrating promising skill for flux estimates in areas without dedicated instrumentation. This study explores atmospheric controls on methane flux estimates across thermokarst and fen landscapes, separated by approximately 4500 km, to better understand carbon cycling in ungauged northern peatland complexes.