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Recent advances in nanoengineering of electrode-electrolyte interfaces to realize high-performance Li-ion batteries
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  • Na-Yeong Kim,
  • Il Gyu Kim,
  • Behnoosh Bornamehr,
  • Volker Presser,
  • Hiroyuki Ueda,
  • Ho-Jin Lee,
  • Jun Young Cheong,
  • Ji-Won Jung
Na-Yeong Kim
University of Ulsan
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Il Gyu Kim
University of Ulsan
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Behnoosh Bornamehr
INM Leibniz-Institute for New Materials gGmbH
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Volker Presser
INM Leibniz-Institute for New Materials gGmbH
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Hiroyuki Ueda
Deakin University
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Ho-Jin Lee
University of Ulsan
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Jun Young Cheong
University of Bayreuth

Corresponding Author:jun.cheong@uni-bayreuth.de

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Ji-Won Jung
University of Ulsan
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Abstract

A suitable interface between the electrode and electrolyte is crucial in achieving highly stable electrochemical performance for Li-ion batteries, as facile ionic transport is required. Recently, intriguing research and development have been carried out to form a stable interface between the electrode and electrolyte. Therefore, it is essential to investigate emerging knowledge and contextualize it. The nanoengineering of the electrode-electrolyte interface has been actively researched both at the electrode/electrolyte and interphase levels, which calls for significant attention. This review presents and summarizes some recent advances aimed at nanoengineering approaches to build a more stable electrode-electrolyte interface and assess the impact of each approach adopted. Furthermore, future perspectives on the feasibility and practicality of each approach will also be reviewed in detail. Finally, this review aids in projecting a more sustainable research pathway for a nanoengineered interphase design between electrode and electrolyte, which is pivotal for high-performance, thermally stable Li-ion batteries.
14 Feb 2023Submitted to Energy & Environmental Materials
16 Feb 2023Submission Checks Completed
16 Feb 2023Assigned to Editor
19 Feb 2023Review(s) Completed, Editorial Evaluation Pending
19 Feb 2023Reviewer(s) Assigned
28 Feb 2023Editorial Decision: Revise Minor
20 Mar 20231st Revision Received
22 Mar 2023Submission Checks Completed
22 Mar 2023Assigned to Editor
22 Mar 2023Review(s) Completed, Editorial Evaluation Pending
23 Mar 2023Editorial Decision: Accept